Variables Affecting Organic Decay Processes In High Tide Pools and Some Effects of This Process in Tigriopus californicus, (Baker 1912) Martin Lynch Hopkins Marine Station Biology 175H Spring 1977 INTRODUCTION The copepod Tigriopus californicus is frequently abundant in high tide pools that have a black sediment and smell of hydrogen sulfide. The sulfide results from the anaerobic decomposition of organic matter, primarily pieces of macroscopic algae, brought to these pools by tidal action. It would appear that oxygen becomes limiting in these isolated marine enviroments due to aerobic decomposition of the same algal ma¬ terial, and the process of sulfate reduction by Desulfovibrio sp.be¬ comes conspicuous. The process of aerobic and anaerobic decomposition affect these enviroments and may in turn have an effect upon other inhabitants such as T. californicus. This study includes a field sur¬ vey of sulphide concentrations found in tide pools of the Central Cal¬ ifornia coastal area, laboratory toxicity studies carried out using T. californicus, and an investigation of the relationships between water depth and sediment depth and their affects on oxygen depletion and sulfide generation during the breakdown of the alga, Macrocystis pyrifera. MATERIALS AND METHODS In the general field survey the area of study was the high tide pools on the Montery penninsula from Mussel Pt. to Asilomar State Beach. Oxygen was measured using a standard Winkler titration (Carritt and Carpenter 1966). Ten milliter samples were drawn off the bottom of the pool just above the sediment with a pipett covered with plankton screening. Great care was exercised in making sure no bottom sediment that might adhere to the screening was washed into the collecting flasks. Samples were placed in 25ml Erlenmeyer flasks and "pickled" immediately with analysis completed within two hours. Sulphide was measured using the colorimetric method described by Strickland and Parsons (Strickland and Parsons 1968). Sulphide samples were collected using a large vol¬ ume turkey baster that was covered with plankton screening. Once again care was exercised in not letting any sediment get in the sample container. Samples were stored in 30ml glass stoppered reagent bottles that were filled to overflowing then stoppered without the inclusion of a bubble of air. Analyses were completed within two hours. pH read¬ ings were taken from the glass stoppered reagent bottles used for sulphide analysis. pH was measured using a Beckman Zeromatic II pH meter. Toxicity studies were carried out using five sulphide concentra¬ tions; 2.5x10-4, 3.Ox10-“, 3.6x10-4, 4.3x10-“, and 5.2x10 M. Solutions were made using filtered seawater and reagent grade Sodium Sulfide and placed in 30ml glass stoppered reagent bottles. Ten animals were added to each bottle. The bottles were filled to the top and stoppered without the inclusion of air. Animals are unaffected by such confinement in plain filtered sea water for periods in excess of one week. Mor- tality was determined and defined as a total lack of movement, even upon shaking. Models of high tide pools were simulated in the laboratory using large 30 x 2.8cm test tubes. Two variables, height of the water colum and depth of sediment were varied while the amount of organic matter was held constant at approximately one gram of Macrocystis. The three water levels tested were 25cm, 15cm, and 5cm. Water height was measured as the distance from the top of the sediment to the top of the water column. Unfiltered seawater from the Hopkins Marine Station seawater system was used. Sediment consisted of coarse beach sand. The sand was washed several times in fresh water to remove organic matter and dried at 60° for one and a half days. Three sediment depths were studied; 1.5cm, 0.5cm, and Ocm sediment. Macrocystis was supplied as circular pieces approximately 2cm in diameter, and weighing approximately I gram. The algal pieces were buried beneath the sediment. To further duplicate conditions in tide pools 10-20 T. californicus were added to each tube. Five replicates were prepared for each set of measurements, thus permitting the daily measurements on undisturbed preparations. Oxygen and sulphide were measured as described above. In addition dissolved interstitial sulphide was determined after thoroughly mixing the sedi¬ ment with the water remaining after samples were taken for oxygen and sulphide in the overlying water. During the period of the measurements the tubes were left open to the air at room temperature in the laboratory. Insoluble sulphide was determined after acidification with 3N HCl. RESULT! Table I shows the oxygen, sulphide, and pH levels encountered in the survey of high tide pools. The highest sulphide level observed was 352 ug/liter. Results from the toxicity studies indicated a minimum lethal dose of 3.0x10 'M sulphide. This concentration corresponds to 10,200ug/liter or thirty times the highest concentration found in the field. Under natural conditions sulphide does not appear to reach levels toxic to T. californicus. However, the isolated tidepools of the high intertidal may be affected in a variety of ways by the periodic input of organic matter in the form of drift algae. Therefore, laboratory simulations were studied in order to elucidate the time course of events including changes in oxygen and sulfide. Two variables appeared most worthy of investigation, ie. depth of sediment and height of water column. Figure I shows the results obtained using a water column of 15cm and three sediment depths; 1.5, 0.5, and Ocm. Looking at figure 1, one sees significantly lower oxygen levels in tubes with sediment while dissolved oxygen in tubes without sediment seem to reach a higher steady state level due to a balance between diffusion and utilization. Between the two sediment levels ther is a significant difference in dissolved oxygen. After fourdays the dissolved oxygen appears to increase in preparations haveng the larger depth of sediment. Another difference between these simulations is the initial rate of oxygen depletion is much faster in tubes with 0.5cm sediment. Figure 2 shows the effects of varying the height of the water column while holding the level of sediment constant at 1.5cm. There is a significantly faster drop in oxygen levels in tubes with shallower sediment indicating that oxygen level is determined by diffusion. This difference in rate of the initial oxygen depletion appears to be related to the size of the initial amount of dissolved oxygen availible. Larger volumes buffer against rapid change. Oxygen in the 25cm column decreases more slowly because of a greater reservoir of oxygen. This buffering by larger volume is also shown by the higher sulphide levels reached in shallower tubes. Another intensity feature is the increase in oxygen occuring with increasing sulphide on day five. This is most dramatic in the shallower tubes. In Figure 3 the height of the water column is held constant while sediment depth is varied. As in figure 1, oxygen drops more rapidly in tubes with less sediment. Also seen in figure 1 but more pronounced here is the difference in oxygen levels for days four and five. For the 1.5cm sediment oxygen increases steadily from day four, this is accompanied by significantly higher sulphide levels than those seen in 0.5cm sediment preparations. In the shallower sediment oxygen levels go below lml/liter on days four and five while sulphide never gets above 64 ug/liter in the interstitial enviroment. Table 2 shows the relative percentages in distribution of sulphide in a water column with the vast majority of sulphide stored as insoluble metallic sulphidesdeposited in the sediment. There is also noticeably more sulphide in the interstitial enviroment in tubes with deeper sediment and less dissolved sulphide in the water column. The total sulphide production in these two simulations is approximately the same. DISCUSSION Chemical changes in the simulations suggest the participation of three microbial populations invilved in the decomposition of organic matter. First a group of anaerobic organisms appear to be involved in the initial breakdown of large polysaccharides in the algal material. This group of microorganisms may also partially oxidize the carbohydrates released by the digestive action. As these more readily utilizable mater¬ ials diffuse from the site of deposition of the algae they become availible to the next group, the anaerobic sulfate reducers dependent upon anaerobic conditions within the sediment. The presence of these organisms is in¬ dicated by the production of hydrogen sulphide. Those materials not utilized by the sulphate reducers diffuse into the water column where the final group of bacteria, the aerobic respiring microorganisms oxidize the nutrients at the expense of dissolved oxygen. Within the time period studied this appears to be dependent on the existence of the initial anaerobic digestive bacteria. The evidence for the importance of these bacteria is shown in figure 1 where anoxic sediment is required for oxygen depletion. This model explains the effects of different sediment depths. In deeper sediment more of the diffusable nutrients would be trapped inside the sediment for use by the sulphate reducing bacteria. As the population of the sulphate reducers increases they would us an increasing proportion of the diffusably nutrients letting correspondingly less material reach the aerobic respiring organisms. As fewer nutrients reach the aerobes their oxygen demands decrease which results in increasing oxygen in the water column. This effect is easily seen in figure 3. Neither of these chemical changes results in a deleterious affect on the enviroment from a chemical point of view. Sulphide never reaches high enough levels to endanger T. californicus. The only possible dele¬ terious effect to T. californicus is the decrease in oxygen near the sediment surface. However, T. californicus can swim to less anoxic water higher in the column. These chemical changes maybe of greater signifi¬ cance in leading to the conversion of macroscopic algae into a form that can be more readily utilized by organisms such as T. californicus which can graze upon the rich microbial flora associated with the organic decay process. ABSTRACT The aerobic and anaerobic decomposition of organic matter in high tide pools and the effects of these processes on Tigriopus californicus was investigated. Changes in dissolved oxygen and sulphide were measured in model prepartions in the laboratory and compared to field measurements. Macrocystis pyrifera was the organic matter used in the study. Water column height and sediment depth were varied to obtain an estimate of the effect of these two variables on aerobic and anaerobic processes. The effects of changing water column with showed an inverse rela¬ tionship where oxygen decreased and sulfide increase as the column height has decreased. The effects of changeng sediment depth showed a direct relationship where oxygen and sulphide levels both increased as sediment depth was increased. The amounts of sulphide in the high tide pools in the field reached levels of 352ug/liter, approximately 1/30 the lethal dose for T. californicus. The importance of this decomposition process to T. californicus is dis¬ cussed. ACKNOWLEDGEMENTS I would like to thank Dr. John Phillips for his invaluble assistance throughout the course of these experiments. LITERATURE CITED 1. Carritt, Dayton E., 1966, Comparison and Evaluation of Currently Employed Modifications of the Winkler Method for Determining Dissolved Oxygen in Seawater; A NASCO Report, J mar Res, 24(3): 286 2. Strickland, J.D.H. and Parsons, T.R., A Practical Handbook of Seawater Analysis, Fisheries Research Board of Canada, Bulletin 167, Ottowa, 1968, p. 41 Table 1: Field Survey of High Tide Pools Pool Oxygen ml/liter Sulphide ug/liter 352 265.6 14.7 11.1 245.8 166 13.6 ——— 6.7 PH 7.8 8.2 8.0 8.9 7.6 1. Ocm sediment 2. Ocm sediment Table 2: Percent Distribution of Sulphide in Simulations* Dissolved S Dissolved S Insoluble S" Water Column Sulfides Interstial Total! 3.4 12.6 84.0 2.2x10° ug/liter 15.9 83.9 2.17x10° ug/liter 0.2 *Values are mean levels from five simulations Figurel: Oxygen levels in simulations with a constant water column of 15cm and varying sediment depth. Bars represent +1 standard deviations. X—x = 1.5cm sediment in ml/liter —□ - 0.5cm sediment in ml/liter -O = 0 cm sediment in ml/liter O— L — O 1 — -O 20— 0 -U¬ o Figure 2: Oxygen and sulphide in the water column, and interstitial dissolved sulphide in simulations with a constant sediment depth of 1.5cm. Bars are + 1 standard deviations. X—x = 0, ml/liter in 25cm water column C— -0, ml/liter in 5cm water column x......x = H,S ug/liter in water column for 25cm column g:::E = H,S ug/liter in water column for 5 cm column x ——x = Interstitial H,S ug/liter in 25cm water column Q——□ = Interstitial H,S ug/liter in 5cm water column —---D-------------- — +-- 10 — 1-----------— +------4- 22 .u 1. . Figure 3: Oxygen and sulphide in water column, and interstitial dissolved sulphide in simulations with a constant water depth of 25cm. Bars are + 1 standard deviations. X—x = 09 ml/liter in 1.5cm sediment Q— -0, ml/liter in 0.5cm sediment x......* = H.S ug/liter in water column in 1.5cm sediment D... = H,S ug/liter in water column in 0.5cm sediment x—— x = Interstitial H,S ug/liter in 1.5cm sediment E--E = Interstitial H,S ug/liter in 0.5cm sediment § x- — — — —x—— 4 r