Heat-Shock Proteins in T. californicus • 2 Abstract The supralittoral harpacticoid copepod Tigriopus californicus is subject to a wide variety of external stressors. Animals were collected from splash pools at Mussel Point, Hopkins Marine Station, Pacific Grove, CA during May 1994 and flash frozen at poolside to examine the expression of HSP60 heat-shock proteins. No correlation was found between HSP60 expression in animals and splash pool salinity, suggesting acclimation through osmoregulation. Differential expression of HSP60 between T. californicus populations, however, was noted. Introduction The harpacticoid copepod Tigriopus californicus, an inhabitant of splash pools at or above the high-tide mark, is subject to wide and largely unpredictable variations in temperature, pH, salinity and water loss. As the high splash pool environment is influenced by erratic meteorological and tidal disturbances, T. californicus must exhibit great tolerance to withstand the daily and seasonal variability of its habitat. The organism is thought employ homeostatic, or at least enantiostatic, mechanisms to enhance its survivability. Recently, the induction of heat shock proteins has been shown to occur in T. californicus in response to extremes of temperature and salinity in the laboratory, suggesting that such proteins may increase the organism's tolerance to adverse environmental conditions in its natural habitat (Ha, 1993; McEvoy, 1993) The heat-shock response, despite its somewhat limiting name, may be elicited by a wide variety of stressors, including anoxia, ethanol, heavy metals, amino acid analogues, inhibitors of oxidative Heat-Shock Proteins in T. californicus phosphorylation, thermal and osmotic fluctuations, and even viral infection (Craig, 1985; Morimoto, et al., 1990). Upon application of a stressor, cultured cells and tissues have been shown to respond by preferentially synthesizing a set of proteins, known as the heat- shock proteins (HSPs), while the synthesis of most other proteins is inhibited or significantly decreased. Production of HSPs may be greatly intensified or even induced de novo, with physiological stress, and thus the heat-shock proteins are identified by their markedly enhanced synthesis, compared to controls, after perturbation (Lindquist, 1986). Furthermore, it appears that the induction of HSPs coincides with the acquisition of resistance to severe stress. In yeast, Saccharomyces cerevisiae, a rapid shift in culture temperature from 23 to 36°C resulted in protection of cells from death at 52°C, a normally lethal temperature for yeast cells (Craig, 1985). Moreover, studies have found that the kinetics of thermotolerance induction and decay are closely correlated with the kinetics of heat-shock protein synthesis and degradation, suggesting that the synthesis of HSPs is the crucial element in the acquisition of tolerance (Lindquist 1986). In the harpacticoid copepod Tigriopus brevicornis, high salinity acclimation was found to enhance the survivability of individuals in a broader range of temperatures (Damgaard and Davenport, 1994). Though the physiological basis for this heterologous tolerance has not been elucidated, it is reminiscent of the numerous stressors capable of inducing the heat-shock response. The stress protein response has been observed in all organisms investigated thus far. Immunological studies have shown heat shock proteins to be among the most highly conserved proteins in nature Though differences exist (Morimoto, et al., 1990; Lindquist, 1986). amongst various organisms, for example in the number of heat- shock proteins and their molecular weights, such conservation in protein sequence suggests that either stress is a universal experience of living creatures, or that the proteins play an essential role in normal physiological processes (Morimoto, et al., 1990; Huey and Bennett, 1990). Yet, while it generally assumed that the HSPs protect • 3 Heat-Shock Proteins in T. californicus cells from adverse environmental effects, the mechanism of their action remains unclear Given the demonstrated ability of T. californicus to tolerate a wide range of adverse environment conditions, it seems appropriate to examine the role the heat-shock response plays in situ. Variation in the heat-shock response was examined at the level of protein synthesis for several unique populations of T. californicus, collected from high tide pools along Mussel Point, Hopkins Marine Station in Pacific Grove, California to provide further insight into the ecological and physiological significance of the stress protein response. Materials and Methods Collection of Tigriopus californicus. Animals were collected with a small strainer consisting of 100um nylon mesh and PVC pipe from high tide pools along the west side of Mussel Point at Hopkins Marine Station in Pacific Grove, California. Animal samplings from each pool were placed in 17 X 100mm polypropylene test tubes, capped, and dropped into a Dewar flask filled with liquid nitrogen for flash freezing. Rock pool temperatures were measured with a Yellow Springs TeleThermometer. Salinity measurements in parts per thousand (%/00) were performed with a American Optics portable refractometer. Water samples from each pool were collected in 35 X 45 mm containers with lids and pH was measured with a Beckman 940 pH meter within 30 minutes. Collection and maintenance of control animals. Animals were collected with a small strainer (see description, supra.), placed in a large beaker containing sea water and carried back to the laboratory Animals were maintained in Instant Ocean artificial seawater (Aquarium Systems, Mentor, ÖH) at 32%/00 or 60%00 and kept in a laboratory incubator with a 12hr light: 12hr dark cycle at approximately 23°C. Animals were fed ground Tetramin (Tetra Sales, Morris Plains, NJ) three times per week and were acclimated for at least 48hr prior to experiments. • 4 Heat-Shock Proteins in T. californicus • 5 Isolation of soluble protein. Prior to protein extraction, flash frozen animals were thawed on ice. Animals were then washed with 2L UV-filtered sea water. Protein samples from each T. californicus population were obtained by grinding whole animals, without regard to sex, in a 2ml Teflon-glass homogenizer (Wheaton Instruments, Millville, NJ) with 200ul homogenization buffer (10ml PBS in lOmM EDTA, 50ul PMSF, 1Oul pepstatin, 1Oul leupeptin, 100ul chymostatin, 50ul NP-40). Homogenate was centrifuged for 10 minutes at 15000 rpm and supernatant removed. Protein concentrations were determined by the method of Bradford using the MicroAssay protocol developed by Pierce Laboratories, Inc. (Rockford, IL). Quantifications were calculated from readings at 595nm from a Beckman DU-7 spectrophotometer. Proteins samples were then mixed 1:1 in 2x solubilizing buffer (8M urea, 4% SDS, 100mM tris, 0.01% bromophenol blue) with dithiothreitol and boiled for 3 minutes. Samples were either used immediately or stored at -20°C. Separation of proteins. Proteins were separated by one¬ dimensional sodium dodecyl sulphate polyacrylamide gel electrophoresis (SDS-PAGE) on 10% minigels (8 X 7 cm) of 1.5mm thickness according to the procedure described by Laemmli (1970) Resolution was at a constant current of 25mA per gel at room temperature. Pre-stained molecular weight standards (Sigma, St. Louis, MO.) were loaded onto each gel for the determination of molecular weights of proteins. Gels not destined for electrophoretic transfer were subsequently stained with Coomassie blue for at least 3 hours and destained overnight in 10% isopropanol and 10% acetic acid. Electrophoretic transfer. Electroblotting of proteins to Immobilon-P PVDF transfer membranes (Millipore, Bedford, MA) was performed according to the procedure described by Burnette (1981) with slight modifications. Following electrophoresis, stacking gel was removed and the resolving gel and two pieces filter paper (Whatman, Hillsboro, OR) were soaked for approximately 5 minutes in transfer Heat-Shock Proteins in T. californicus • 6 buffer (49.6 mM tris, 384mM glycine, 20% methanol, 0.01% SDS ) Immobilon was soaked approximately 5 minutes in methanol. Gel and Immobilon were mounted in a Hoeffer TE22 transfer apparatus between the two pieces of Whatman filter paper. Transfer was carried out at 25mA constant current for 12 hours at 4°C. Immunostaining. Äfter transfer, Immobilon membranes were removed from the gel and blocked with TBS/Milk/Tween (60ml 5X TBS, 15g Carnation nonfat dry milk, 0.3ml Tween20) for 1 hour at 37°C. Blots were subsequently washed with TBS/Tween (IX TBS, 0.5% Tween) for 15 minutes. Probing occurred with Rabbit Anti-HSP60 polyclonal antibody, developed against Synechococcus sp. (cyanobacteria) (StressGen, Victoria, B.C., Canada) in 1:1000 dilution in TBS/Milk/Tween at room temperature for 1 hour with rapid rocking. Following primary antibody incubation, blots were rinsed for 10 min in IX TBS, 10 min in TBS/Tween and 10 min in IX TBS Secondary antibody probing occurred with anti-rabbit IgG (whole molecule) peroxidase conjugate (Sigma, St. Louis, MO) diluted 1:1000 in IX TBS for 1 hour with rapid rocking. Äfter rinsing, blots were incubated in Renaissance wester blot chemiluminescence reagents (DuPont NEN, Boston, MA) for 1 minute and imaged on Kodak X¬ OMAT AR film. Densitometric analysis. Wet gels and X-ray photographs of immunoblots were scanned by transmittance with a green filter using a Pharmacia ImageMaster DTS and analyzed with Pharmacia ImageMaster Software (Version 1.0) according to prescribed methods. Results In the field at Mussel Point, salinity in the high tide pools inhabited by Tigriopus californicus varied from 15 to 88%00 during the period of experiments. The most saline rock pool (88%0) in which T. californicus was found completely evaporated after Heat-Shock Proteins in T. californicus approximately 1 week of observation. An independent population of T. californicus from this pool did not revive after the next rainfall, as the subject pool became networked with a neighboring pool of lesser salinity. Temperatures recorded in pools inhabited by T. californicus ranged from 12.1 to 27.2°C. Low pool temperatures generally were produced rapidly by rare periods of high wave activity, which happened to largely wash out high rock pools long detached from the sea. During these periods of high tides, salinity in the various pools was noted to return rather quickly to that of the ocean (ca. 33%00) High tides also had the effect of depleting the population of T. californicus in some pools, but most populations appeared to recover within several days. Figure 1 shows a immunoblot, probed for HSP60, for several unique populations of T. californicus after equal loading for total protein (20ug). Laboratory controls at 32%00 and 60%0 appear in lanes 1 and 2, respectively, numbered left to right. Lanes 3 through 8 represent T. californicus flash frozen at poolside for various splash pools, with salinities ranging 33 to 78.7%0, increasing left to right along the blot (see Table 1). Note that neither temperatures nor pHs were constant during these samplings, but these parameters were deemed not significantly different as salinities. Prominent reaction of the anti-HSP60 polyclonal antibody occurs with protein(s) of approximately 58kD. Note some anti-HSP60 cross-reactivity occurs with lower molecular weight proteins in certain populations, particularly in lanes 3 and 6. Densitometric analysis of the 58kD bands is shown in Figure 2. Trace densities (O.D. X mm) for these bands are listed in Table II. Trace densities are linearly proportional to quantity of antigen present, provided antigen-antibody interactions are quantitative in the presence of excess antibody (Fernández and Kopchick, 1990). Protein in lanes 6 and 8 were obtained from T. californicus in the same rock pool, sampled at different times—when salinities were measured at 60% and 78.7°/00, respectively. It appears that significantly more HSP6O is produced in the T. californicus population from this pool, over control levels and over levels obtained for other Heat-Shock Proteins in T. californicus • 8 populations. Lanes 4 (43.2%0), 5 (51.9%0), and 7 (78.7%00), representing animal samples obtained from unique splash pools, have approximately equal levels of HSP60 protein(s) at 58kD. Lane 3, corresponding to a sampling from a 33%00 rock pool, appears to be somewhat anomalous, perhaps due to underloading. Discussion The levels of HSP60 production under increased salinities in in situ populations of Tigriopus californicus were found to be different than those determined by acute salinity shock experiments performed in the laboratory by Ha (1993) and McEvoy (1993). Ha found that when T. californicus was acclimated at 16.5%0 artificial seawater for 24hrs and then immediately transferred to 66%0 seawater, dramatic induction of HSP60 and HSP7O occurred. Ha further noted that the level of heat-shock proteins in individuals declined to "pre-shock" levels after approximately four hours at 66%o. In concordance, Hakimzadeh and Bradley (1990) found a gradual return to normal (non heat-shock) proteins after severe heat shock in the copepod Eurytemora affinis. Since the heat-shock response appears to be transient, differences in findings may be related to acclimation time. In the wild, animals are rarely, if ever subjected such rapid hyperosmotic shock, as evaporative processes occur over a much greater time scale. Since approximately equal amounts of HSP6O at 58kD were found among the different populations at varying salinities (Pool Z, 43%0; Pool D, 51%00; Pool Y, 72%/0), it may be that T. californicus copes with a hypersaline environment without maintaining higher basal levels of HSPs. An extension of this finding is the prediction that species which live and function in more stringent habitats (such as hypersaline environments) have higher thresholds for HSP induction. Though studies have shown that the kinetics of thermotolerance induction and decay closely coincide with the kinetics of heat-shock protein synthesis and degradation (Lindquist, 1986), there is some evidence that tolerance is independent of HSP Heat-Shock Proteins in T. californicus induction. Easton, et al. (1987) found in the salamander Eurycea bislineata that heat hardening (the ability to withstand higher maximum temperatures with repetitive treatments) occurred regardless of whether HSP synthesis was induced. Thus it appears that acclimation to stringent conditions may be independent of heat shock protein synthesis. The source of T. californicus euryhalinity may then be related to its ability to osmoregulate its intracellular solute pool. Burton and Feldman (1982) found that during hyposmotic stress, the concentration of free amino acids within the body homogenate of individuals significantly decreased in 3 to 5hrs. Under hyperosmotic stress, free amino acid concentration was found to increase within 3hrs. Remarkably, as little an increase as 2%/00 has been shown to be sufficient to induce proline synthesis in animals acclimated to seawater at 16.5%0 (Burton, 1991). Thus in the wild, where gradual salinity changes are commonplace, it appears that T. californicus may maintain homeostasis by osmoregulation rather than by exhibiting a stress protein response. This does not explain, however, why some populations of T. californicus exhibit consistently greater concentrations of heat-shock Animal populations in Pool X, sampled during proteins than others. two distinct periods in this study (at 60%00 and 78.7°/00), appeared to express more HSP60 than other pools. The reasons for this are unclear. Perhaps the inhabitants of this pool, as a distinct population with unique genetic characteristics, simply express higher basal HSP60 expression. Additionally, we may not rule out the possibility that increased synthesis is the result of a stressor for which we did not account. However, this latter possibility seems unlikely, given Variation in Pool X’s proximity to other pools included in this study. the level of HSP60 production was also observed between control animals at 32%0 and 60%/00, obtained from different populations. Comparison of stained gels for the various populations indicates that protein composition varied somewhat from group to group. Certain bands appeared more intense in some populations compared to others. In some cases, unique bands were observed for a given population. The explanation for this remains unclear. Perhaps true • 9 Heat-Shock Proteins in T. californicus genetic differences exist between populations. Variation in protein composition may also be related to the unique physico-chemical environment of each pool. Alternatively, differences may be artificially exaggerated due to fallible sampling techniques. Nimkin (1977) found a significant positive association of salinity and percent females in high saline pools. Female copepods apparently are more resistant to stressors than males (Hakimzadeh, et al., 1990; Damgaard, et al., 1994). If sex ratios are truly different amongst the various splash pools tested, then a sampling error may have occurred, as no attempt was made to separate males and females prior to homogenization. This possibly accounts for observed protein differences across populations. In any case, if different populations of T. californicus have different protein compositions, it may be unwise to weigh animals based on total protein concentration. For example, suppose two hypothetical populations (« and B) of T. californicus produced identical amounts of HSP6O. But suppose population a had twice as much blunderin (a hypothetical 116kD protein that serves no purpose) as population ß. If we load the lanes of our gel for equal total protein, transfer protein to a nylon membrane and then probe for HSP60, population B would appear to have more HSP60 than population a. A new method of weighing the animals must therefore be developed. Counting individual animals may be the best alternative. However, the problem of variability in chemical composition amongst individuals would remain. We would also be introducing a new factor—individual variability in body size. Another obstacle to unambiguous, definitive results is the fact that this study was conducted in the field. Thus it was not possible to easily measure the effect of one variable while holding all others constant. In the future, it may be more productive to devise splash pool models in which variables may be controlled. • 10 Heat-Shock Proteins in T. californicus° 11 Conclusion The degree of conservation of HSPs and the heat-shock response across species implies strong natural selection. Since natural selection can only act on the stress response when it is evoked, stress which induces HSPs must be somewhat common among individual organisms. We have sampled Tigriopus californicus from rock pools of various salinities and measured the expression of HSP60 in animals. No correlation was found between HSP60 expression in animals and pool salinity, apparently because of the ability to osmoregulate. However, differential production of HSP60 was noted among distinct T. californicus populations. Whether these differences are genetic or phenotypic remains to be elucidated. Acknowledgments I am grateful to Dr. R. Paul Levine for his guidance and everlasting commitment to this project. Additional thanks go out to Dr. Mark Denny and Dr. Jim Watanabe for providing me with the means to carry about the field work associated with this study. Thank you to Dr. Jan von Kampen, Sunny Sanders, and Dr. Virginia Weis for taking time out of their busy schedules to assist me and for their steadfast patience and support. Literature Cited Burnette, W.N. (1981). "Western blotting: Electrophoretic transfer of proteins from sodium dodecyl sulfate-polyacrylamide gels to unmodified nitrocellulose and radiographic detection with antibody and radioiodinated protein A. Analytical Biochemistry, 112:195-203. Heat-Shock Proteins in T. californicus° 12 Burton, R.S. (1991). "Regulation of Proline Synthesis During Osmotic Stress in the Copepod Tigriopus californicus:" Journal of Experimental Zoology, 259: 166-173. Burton, R.S. and M.W. Feldman. (1982). "Changes in Free Amino Acid Concentrations During Osmotic Response in the Intertidal Copepod Tigriopus californicus. Comparative Biochemistry and Physiology, 73A: 441-445. Craig, E.A. (1985). "The Heat Shock Response." CRC Critical Reviews in Biochemistry. Volume 18, Issue 3. Damgaard, R.M. and J. Davenport. (1994). "Salinity tolerance, salinity preference and temperature tolerance in the high- shore harpacticoid copepod Tigriopus brevicornis. Marine Biology, 118:443-449. Easton, D.P., P.S. Rutledge, and J.R. Spotila. (1987). "Heat shock protein induction and induced thermal tolerance are independent in adult salamanders." Journal of Experimental Zoology, 241: 263-267. Fernández, E. and J.J. Kopchick. (1990) "Quantitative Determination of Growth Hormone by Immunoblotting. Analytical Biochemistry, 191: 268-271. Ha, C.M. (1993). "Stress Induced Heat Shock Proteins in Tigriopus californicus. Unpublished manuscript on file at Hopkins Marine Station Library, Stanford University, in Final Papers, Biology 175H. Hakimzadeh, R. and B.P. Bradley. (1990). "The Heat Shock Response in the Copepod, Eurytemora Affinis (Poppe)." Journal of Thermal Biology. 15: 67-77. Huey, R.B. and A.F. Bennett. (1990). "Physiological Adjustments to Fluctuating Thermal Environments: An Ecological and Evolutionary Perspective." In R.I. Morimoto, A. Tissières, and C. Georgopoulos (Eds.), Stress Proteins in Biology and Medicine (pp. 37-59). New York: Cold Spring Harbor Laboratory Press. Heat-Shock Proteins in T. californicus° 13 Laemmli, U.K. (1970). "Cleavage of structural proteins during the assembly of the head of bacteriophage T4. Nature, 227: 680- 685. Lindquist, S. (1986). "The Heat-Shock Response", Annual Review of Biochemistry, 55:1151-91. MCEvoy, T.A. (1993). "Identification and Induction of Heat Shock Proteins in Tigriopus californicus. " Unpublished manuscript on file at Hopkins Marine Station Library, Stanford University, in Final Papers, Biology 175H. Morimoto, R.I., A. Tissières, and C. Georgopoulos. (1990). "The Stress Response, Function of the Proteins, and Perspectives." In R.I. Morimoto, A. Tissières, and C. Georgopoulos (Eds.), Stress Proteins in Biology and Medicine (pp. 1-36). New York: Cold Spring Harbor Laboratory Press. Nimkin, K. (1977). "Differential Mortality to Salinity Stress and its Relation to Sex Rations in the Marine Copepod, Tigriopus californicus." Unpublished manuscript on file at Hopkins Marine Station Library, Stanford University, in Final Papers, Biology 175H. Table I Sampled Pools MNNNNNNNNNN Salinity ( Sa ) Temperature (C) 8.00 Laboratory Control 32.0 23.0 8.00 60.0 Laboratory Control 23.0 Pool A 17.0 8.76 9.01 43.2 17.0 Pool Z 51.9 8.74 Pool D 18.2 60.0 8.87 Pool X 9.11 19.5 Pool Y Politn ad Table II HSP60 Trace Densities for T. californicus Populations (Band at 58 KD) soscoceosesssssossesesesseeesssesssssssseessessocosoeeeesesssoooesse Sample Trace Density (OD X mm) 1.958 Laboratory Control 1.226 Laboratory Control 0.279 Pool A 1.602 Pool Z 1.429 Pool D 2.459 Pool X Pool Y 1.503 mnen e: Band quantification is performed as follows: Average optical density of each row of pixels is calculated across sample width (horizontally). Average optical density for each pixel row is then integrated over the band height (vertically). This gives the dimensions OD X mm. List of Figures Figure 1. Western blot with anti-HSP60 polyclonal antibody probe. Samples obtained from various Tigriopus californicus populations at Mussel Point. Twenty (20) ug samples of soluble protein derived from laboratory animals maintained in 32%0 and 60%00 seawater were loaded in lanes 1 and 2, respectively (numbered left to right). Soluble protein (20ug) derived from in situ populations was loaded in lanes 3 through 8. Order of these lanes, left to right, is as follows: Pool A (33%/0), Pool Z (43.2%/0), Pool D(51.9%0), Pool X(60%/00), Pool Y(72.8%0), and Pool X(78.7%/0). Prominent reaction occurs with protein(s) at 58kD. Note cross-reactivities in lanes 3 and 6. Figure 2. Histogram representing densitometric analysis of 58kD band from Western blot. Units along the ordinate are O.D. X mm (trace density). Animals of Pool X (lanes 6 and 8) apparently produce higher levels of HSP60. 8 a 3 8