ADDITIONAL INFORMATION, IF ANY, CONCERNING AUTHORS, ADDRESS, TITLE, OR CITATION DATA PLEASE TYPE ABSTRACT DOUBLE SPACED BELOW Beppu, William J. (Hopkins Marine Station of Stanford University. Pacific Grove, California). A Comparison of Carbohydrate Capabilities in Four Species of Acmaea (Mollusca: Gastropoda; Prosobranchia). The Veliger The carbohydrate digestion of four limpets, Acmaea scabra, A. digitalis, A. limatula, and A. scutum was studied. The presence Kagt of a -carrageeninase, andagarase, a laminarinase, a fucoidinase. an alginase, and an amylase was found in all species. Someohydrase correlation of available sources of food with enzyme activity was found. Carbohydrase levels in starved animals were compared with levels in non-starved animals. A decrease in enzyme activity during starvation was found, and the amount of this decrease could be correlated with height in the intertidal, higher species (A. scabra and A. digitalis) showing less decrease than lower species (A. limatula and A. scabra). This correlation might be related to food retention time and to feeding behavior.-Author. PLEASE DO NOT TYPE BELOW THIS LINE 62 CALBOIRDRAT CAPABILTTIES COMPARIS IN FOUR SPECIES OF ACMAEA Gastropoda: Prosobranchia llusca: william J. Beppu Hopkins Marine Station of Stanford Univers Pacific Grove, California William J. Beppu An examination of the distribution of the genus Acmaea in the intertidal revealed that the various species have their highest population densities in different tidal zones. One of the characteristics of these zones is a dif- ference in their algal flora. These various intertidal algae, which synthesize a variety of polysaccharide mate- rials (see Peat and Turvey, 1966) constitute a potential source of food to herbivorous scrapers such as Acmaea. ess at The assimilation of these materials would require a varie carbohydrases and led to the present comparative study of the carbohydrases present in the digestive tracts of four species of Acmaea. MATERIALS AND METHODS The species chosen for this study were: Acmaea abra (Could, 1846); A. igitalis Eschscholtz, 1833; A. limatula Carpenter, 1864; and A. scutum Eschscholtz, 1833. Large representatives of these species were collected from areas of their maximum population density at Pescadero Point, Monterey County, California. To remove the digestive tract, the animals were anaesthetized in isotonic magnesium chloride isotonic with seawater, and the entire digestive tract along with associ- ated glands (digestive gland, buccal salivary gland, and William J. Beppi esophageal salivary gland) excised and placed in 37 sodium chloride in an ice bath. An enzyme extract was prepared, containing 1 part tissue, 8 parts 36 sodium chloride, and 1 part of a saturated solution of ovomucoid (ovomucoid dis- olved in either 0.1 Macetate buffer, ph 5.5, or 0.1 M Tris puffer, ph 7.2). This mixture was homogenized in a tissue grinder and then centrifuged for 30 seconds at half maximum speed in an International Clinical Centrifuge. Ovomucoid, prepared by the method of Fredericq and Deutch (1949), was used as an inhibitor of proteolytic enzymes since initial experiments indicated low carbohydrase activity, possibly resulting from degradation of the enzymes by proteolysis. of ovomucoid permitted detection of higher levels of anzyme activity, and was therefore used in all reported periments. One ul of ensyme extract was incubated with l ml of polysaccharide solution in 3 ml of buffer. Two buffers were used, either 0.1 M acetate at pli 5.5,or 0.1 M Tris at p 7.2. The polysaccharides included in this study were arch (Baker and Adamson, Reagent grade), agar (Difco), arrageenin Kappafraction) isolated from Rhodoglossum spp. and laminarin, fucoidin, and alginic acid isolated from . The mixtures were incubated for 1 hour at vetia 200C. Enayme and substrate controls were similarly incubated Liam J. Bepu All tubes, including enzyme and substrate controls, were layered with toluene as a bactericide, after Galli (1956 At the end of the incubation period enzyme activity was stopped by sodium hydroxide-zinc sulfate precipitation, and aliquots were assayed for reducing sugar by a modifica- tion of Nelson's procedure (1944). This modification was he substitution of sodium hydroxide for barium hydroxide prevent precipitation of sulfated oligosacharides formed during enzymatic hydrolysis of K-carrageenin and fucoidin. The optical density of the final solution was measured in a Klett-Summerson photoelectric colorimeten using a green filter. Nwo standard glucose solutions, 1509 and 509, were run with each set of assays, and all readings were evaluated by comparison with a glucose standard curve. Values represent an average of two deter minations of total reducing sugar released in the incubation mixture, and correspond to the activity of 0.1 ml of tissue xtract. The assay was found to be reproducible within 10 percent. The minimum value considered to be significant in the tables was taken to be 50 ug. REs Algal associations: To correlate diet with digestive activity, a rough survey was made of the collection area. Heights for maximum Lliam J. 5 concentration of larger specimens were estimated as 5 ft for Acmaea scabra, 4 ft. for A. digitalis, 3 ft. for A. limatula, and 2.5 ft. for A. scutum. Algae growing in the spective collection areas were: A. scabra, microscopic lgae only; A. digitalis, microscopic algae, Ralfsia spp., and some Peysonnelia spp.; A. limatula, microscopic algae, Sigartina spp., Endocladia spp., and Pelveti- Balfsia s . andA. scutum, microscopic algae, Ralfsia spp., Sigartina spp., and Porphyra spp. The microscopic algae ir this area were varied green and red algae (Haven, 1966). his is not meant to be a definitive list of the dietary onstituents of these animals, but rather an observation of the algae available for food in the limited areas from which the organisms were collected. Enzyme activit In the first experiment, the animals were "starved" in an aquarium scraped free of algae, and kept in the dark. After 4-6 days of starving, extracts of the gut were made, and ensyme activity determined. The results are recorded in Table 1. The results show the presence of a powerful amylase with higher activity at ph 5.5 in all'species. An alginase was also demonstrated in all species. All species examined William J. B. xcept Acmaea limatula exhibited a fucoidinase with highes activity at pH 5.5. Small amounts of agarase and laminari- nase were found in A. scutum, A. scabra, and A. digitalis a K-carrageeninase also being present in the two latter digitalis and A. scabra show the greatest species. overall activity, with sionificant amounts of enzyme activi demonstrated for all substrates tested. na second experimental series, animals were col lected fresh from the field and extracts prepared within Enzyme activities determined are shown in three hours. Table 2 powerful amylase was again evident, but wit these animals small amounts of activity for all substrate digitalis showed the were found in all species. Acmae. greatest overall activity. comparison of the starved animals with the non- tarved animals shows, in general, greater activity in non ved animals. However, some species differences are ident Although there are some deviations for particular ubstrates, there is a general grouping in the effect of tarvation, starvation causing a much greater decrease in activity in Acmaea limatula and A. scutum than in A. scabra and A. digitalis. Amylase activity was particularly affected. William J. Beppu 6 DISCUSSION Green and red algae, which contain starches, K-carrageenin, and agar (Peat and Turvey, 1965), are available to all species of Acmaea studied, and the high recorded amylase activity correlated well with this. Brown algae, containing alginic acid, fucoidin, and laminarin (Peat and Turvey, 1965), are available to all species except A. scabra. Although this correlates well with the low alginase activity found in A. scabra, it is not reflected in the laminarinase or fucoidinase activity. Eaton (1966) has made a careful study of the diet of A. limatula and A. pelta. A similar study of the other species would be desireable. The data on changes in carbohydrase activity due to star¬ vation suggest that the degree of these changes is a function of height in the intertidal zone, higher species (Acmaea scabra and A. digitalis) showing loss drop in activity than lower species (4. limatula and 4. scutum). Two possible reasons for this difference are food retention time and feeding behavior. In fresh animals, the lower species oliminated food that was only partly digested at a much greater rate than the higher species. In the starved animals, the remains of well-digested food were still found in the gut of the two higher species, whereas nothing was found in the gut of the two lower species. This difference in food retention time correlates well with the changes in enzyme activity during starvation. The feeding behavior of tho higher species has also been found to be more sporadic than that of the lower species. The lower species, being splashed or under water a greater amount of the tine than the higher species, are thus able to move and feed for longer periods of time. Trus the higher species must 68 William J. Beppu retain and digest food more efficiently, as was found, and are therefore, not as susceptible to the effects of deprivation of food. SUMARY The carbohydrate digestion of four limpets, Acmaea scabra, A. digitalis, A. limatula, and A. scutum was studied. The presence of a K-carrageeninase, an agarase, a laminarinase, a Tucoidinase, an alginase, and an amylase was demonstrated for fods avaae all species. Some correlation of with enzyme activity was found. Carbohydrase levels in starved animals were compared with levels in non-starved animals. A decrease in enzyme activity during starvation was found, and the amount of this decrease could be correlated with height in the intertidal, higher species (A. scabra and A. digitalis) showing less decrease than lower species (A. limatula and A. scutum). This correlation might be and related to food rotention time feeding behavior. ACKOLEDG My sincere thanks to Dr. John H. Phillipps for purified samples of algal polysaccharides and for his guidance during the entire study. Many thanks to Dr. David Epel for his great assistance in preparing this paper. This work was made possible by Grant GY806 from the Undergraduate Research Participation Program of the National Wcience Foundation. 7 64 O William J. Beppu 8 LITERATURE CITED Eaton, Charles 1966. The Activity and Food of the File Limpet, Acmaea limatula. The Veligen, this volume. Frederice, Eugene & H. F. Deutch- 1949. Studies on ovomucoid. Journ. Biol. Chem 181: 499-509 Galli, Donald Richard 1956. Carbohydrate digestion in an herbivorous marine snail, Terula funebralis. Haster of Arts Thes., Stanford Univ.; 153 pp. Haven, Stoner 1966. Personal communication Nelson, Norton 1944. A photometric adaptation of the Somogyi method for the determination of glucose. Journ. Biol. Chem. 153: 375-380 Peat, Stanley & J. R. Turvey 1965. Polysaocharides of marine algae. Pp. 1-45, Progress in the chemistry of organic natural products, v. 23. New York Wien & Springer-Verlag viii-397 pp., 58 fig. 70 page 1: Footnotes Permanent Address: William J. Beppu William J. Beppu 72 Aelt 1 Carbohydrase Activity of Starved Animals kkak Substrates Opecies pH Fucoidin Alginic Acid Agar Laminarin K- rageenin Starch Total Reducing Sugar Released in 1 Hour - e 5.5 65.8 ug 32 ug 197A 1324g 19748 3520 ug A. scabra 43.9 7.2 109 1530 168 298 298 224 3420 5.5 112 A. digitalis 55.9 1440 7.2 2760 20.8 A. limatula 5.5 811 239 7.2 82.0 82.0 61.5 1660 103 5.5 41.0 A. scutum 681 7.2 Opecies A. scabra A. digitali A. limatula A. scutum l William J. Beppu 78 19812 2 Carbohydrase Activity in Non-Starved Animals — Substrates pI K-carrageenin Laminarin Fucoidin Alginic Acid Starch Total Roducing Sugar Released in 1 Hour 128 ug 5.5 51.4g 77.0Ag 51.4Ag Opg 3440 gg 7.2 77.0 1980 100 250 275 225 3850 25.0 150 100 7.2 1950 51.4 103 103 103 51.4 5.5 3680 O 7.2 206 1870 5.5 300 198 175 150 150 3320 125 50.0 100 7.2 50.0 1775