C O SIX UNKNOWN GREEN PIGMENTS FROM MOLLUSKS PATRICIA MCGEE JUNE 4, 1964 Dr. JOHN PHILLIPS HOPKINS MARINE STATION The unknown green pigment from Tegula funebralis and the similar green pigments from Tegula brunnea, Tegula montereyi, Tegula pulligo, the red and black abalone (Haliotis) are the pigments under study. The unknown green pigments were extracted with methanol in all cases. The procedure of extraction and removal of the carotenoid contaminations are as follows: The gonad of the organism is removed and placed in a waring blender with 100% methanol. The supernatant from this process is then centrifuged to remove all the tissue particles. This solution is taken to dryness on a vacuum distiller at not more than 40°C. The pigments are then redissolved in water. The aqueous solution is then partitioned with anhydrous ether; the green pigment remains in the aqueous phase and the carotenoids move to the ether phase. Thi process is repeated with fresh ether until the yellow color in the ether has disappeared. The aqueous green pigment is then taken to dryness and redissolved in distilled water two times. The pigment in this state is what I refer to as the crude pigment. The absorption spectra of the pigments in this stage are provided in the attached sheets. The pigments, in all cases, were observed to have the characteristics of pH indicators after the pH was initially taken to 11. At pH 11, a precipitation is formed. This precipitation was found to be soluble in distilled water at pH 4 to 6. A similar precipitation may also be obtatined by addition of acetone to an C aqueous solution of the crude pigment. This precipitate was also soluble in water, and in Tegula funebralis, by a Folin protein test it indicated that thereis 3.6mg of protein per ml of "standard' solution of crude pigment. The pigments were all pH indicators in the alkaline range. They all appeared yellow to orange, depending on concentration, at pH 9.5. The spectra of the pigment from Tegula brunnea in the acid and alkaline states appears in the attached sheets. The exact turning point of the T. brunnea was determined at 8.3 pH. All the pigments were observed to be reduced by the addition of Nag S2 O (sodium hyposulfite). The pigments, however, could not be induced to reoxidize by addition of sodium peroxide or auto-oxidation by bubbling with air. An attempt was also made to reduce the pigments under the less severe conditions of anoxia by nitrogen bubbling through them. This was unsucessful. In the case, of Tegula funebralis it was calculated that it takes 5.7x102 M sodium hyposulfite to reduce the pigment to the yellow state. It is noted that upon reduction the visible peak at 650mu is removed; however, the ultra violet peaks at 271 and 325mu remain the same. (the absorption spectra are included). The configuration of all the spectra of these various pigments are similar; however, the absorption peaks vary within a range of 4Omu in the visible and 2 to 10mu for th UV peaks. It would seem that perhaps the compounds are members of the same family. This asumption is further supported by identical solubilities and behavior toward hydrogen ion concentration. Absorption Spectra TEGULA FUNEBRALIS TEGULA BRUNNEA TEGULA MONTEREYI PEGULA PULLIGO RED ABALONE BLACK ABALONE Solubilities TEGULA FUNEBRALIS TEGULA BRUNNEA TEGULA MONTEREYI TEGULA PULLIGO RED ABALONE BLACK ABALONE of Crude Pigments 650 325 271mu 640 330 271mu 610 330 271mu 610 330 271mu 610 330 270mu 610 320 270mu Ho0, acet., MEOH., ETOH SAME SAME SAME SAME SAME 153 1 . aa- 8 8 o 6 384 8 5 J3e N t S 156 85 88 85 8 § H + 5. 157 ) S o ES S N